Researchers develop mechanism of electrical 180° switching of Néel vector in spin-splitting antiferromagnet

A research team led by The Hong Kong University of Science and Technology (HKUST) and Tsinghua University has theoretically proposed a new mechanism of electrical 180° switching of Néel vector and experimentally realized it in antiferromagnetic materials with spin-splitting band structure featuring the C-paired spin-valley locking, also referred to as an altermagnet. The team also demonstrated the material's capability to manipulate Néel vector, paving the way for the manufacturing of ultrafast memory devices.

The study is published in Science Advances.

Antiferromagnetic spintronics has sparked widespread interest due to its enormous potential for creating ultra-dense and ultrafast antiferromagnetic memory that is suitable for modern high-performance information technologies.

The electrical 180° switching of the Néel vector is a long-term objective for producing electrically controllable antiferromagnetic memory using opposite Néel vectors as binary "0" and "1." However, the state-of-art antiferromagnetic switching mechanisms have long been limited to 90° or 120° switching of Néel vector, which unavoidably requires multiple writing channels that contradict ultradense integration.

The study of electrical 180° switching of Néel vector makes spin-splitting antiferromagnet a new potential candidate for ultrafast memory.

Specifically, in collinear antiferromagnet, the Néel vector n has two stable states: n₊ and n_- with symmetric energy barriers. To leave an asymmetry of energy barriers, the team led by Prof. Liu Junwei, Associate Professor at the Department of Physics at HKUST proposed to exert an external magnetic field to interact with the tiny DMI-induced moment.

Then, the damping-like spin-orbit torque can be used to drive Néel vector n to cross the barrier from n₊ to n_- but cannot cross the opposite one (Figure 1a). As shown in Figure 1b, the atomic spin model simulation shows that n can be deterministically switched to state n₊ or n_- in 0.1 ns. Integrating the non-zero Berry curvatures on spin-splitting bands of tight-binding model, the anomalous Hall conductivities show high sensitivity to these two states n₊ and n_-, shown in Figure 1c.

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In experiments led by Prof. Pan Feng and Prof. Song Cheng, from the School of Materials Science and Engineering at Tsinghua University, the good cyclic performance of fabricated antiferromagnetic Mn5Si3 thin film is shown in Figure 1d, which means the current-driven 180° switching of Néel vector is robust and sustainable.

In fact, the team had presented a new theory as C-paired spin-valley locking (SVL) a few years ago in Nature Communications, indicating a new way to induce the magnetization in antiferromagnet and laying the foundation of switching of Néel Vector.

Compared to conventional T-paired SVL materials, the C-paired SVL materials create the spin-splitting bands by the strong exchange coupling between itinerant electrons and local magnetic moments instead of SOC.

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Furthermore, the spin-splitting valleys are paired with opposite spin directions by preserved crystal symmetry rather than time-reversal symmetry, as shown in Figure 2. In practice, a strain / charge current can be exerted to slightly break or affect the crystal symmetry and therefore induce a net magnetization / noncollinear spin current.

Based on the theoretical and experimental study of electrical 180° switching and readout of the Néel vector in Mn₅Si₃, electrical-controllable AFM memory devices are available with High efficiency and high reproducibility. This basic work achieved the information transformation between charge and spin degrees of freedom in antiferromagnet, paving the way for the rapid development of spintronics in electronics industry.

With its potential application as a storage device, such as in a computer hard drive, the material presents notable benefits including enhanced read and write speeds, as well as increased storage density.

In the future, Prof. Liu hopes that the team will explore more switching mechanisms and the underlying physics, and try to search for more suitable material platforms with higher efficiency.