The path length of light in opaque media

November 10, 2017, Vienna University of Technology
Light on its way through a liquid: In case of a transparent liquid (left) light paths are straight lines. In case the liquid is made opaque through nanoparticles (right) light paths get more complicated through scattering. Some of the paths become longer, others shorter - on average though the length of light paths is the same as in the transparent case. Credit: Vienna University of Technology

A seemingly paradoxical prediction in physics has now been confirmed in an experiment: No matter whether an object is opaque or transparent, the average length of the light's paths through the object is always the same.

What happens when light passes through a glass of milk? It enters the liquid, is scattered unpredictably at countless tiny particles and exits the glass again. This effect makes milk appear white. The specific paths that the incident light beam takes depend, however, on the opacity of the liquid: A transparent substance will allow the light to travel through on a straight line, in a turbid substance the light will be scattered numerous times, travelling on more complicated zig-zag trajectories. But astonishingly, the average total distance covered by the light inside the substance is always the same.

Professor Stefan Rotter and his team (TU Wien, Austria) predicted this counter-intuitive result together with French colleagues three years ago. Now he and his collaborators from Paris verified this theory in an experiment. The results have now been published in the journal Science.

Particles and Waves

"We can get a simplified idea of this phenomenon when we imagine light as a stream of tiny particles," says Stefan Rotter. "The trajectories of the photons in the liquid depend on the number of obstacles they encounter."

In a clear, completely transparent liquid, the particles travel along straight lines, until they leave the liquid on the opposite side. In an opaque liquid, however, the trajectories are more complicated. The beam of light is scattered frequently along its way, it changes its direction many times, and it can only reach the opposite side after covering a long distance inside the opaque substance.

Simulation results for light paths in circular areas with different degrees of opacity. Light comes in from the left with many different injection angles. Credit: Romain Pierret & Romolo Savo

But in a turbid liquid, there are also many photons, which will never reach the opposite side. They do not completely traverse the liquid, but just penetrate a little below the surface and after a few scattering events they exit the liquid again, so their trajectories are rather short. "It can be shown mathematically that, rather surprisingly, these two effects exactly balance," says Stefan Rotter. "The average path length inside the liquid is thus always the same—independent of whether the liquid is transparent or opaque."

At second glance, the situation is a bit more complicated: "We have to take into account that light travels through the liquid as a wave rather than as a particle along a specific trajectory," says Rotter. "This makes it more challenging to come up with a mathematical description, but as it turns out, this does not change the main result. Also if we consider the wave properties of light the mean length associated with light penetrating the liquid always stays the same, irrespective of how strongly the wave is scattered inside the medium."

Experiments in troubled water

The theoretical calculations describing this counterintuitive behaviour have already been published three years ago in a joint publication by Stefan Rotter's team and his colleagues from Paris. Now the same research groups managed to verify the remarkable result in an experiment. Test tubes were filled with water, which was then obfuscated with nanoparticles. As more nanoparticles are added, the light is scattered more strongly and the liquid appears more turbid.

"When light is sent through the liquid, the way it is scattered changes continuously, because the nanoparticles keep moving in the liquid," says Stefan Rotter. "This leads to a characteristic sparkling effect on the tubes' outer surface. When this effect is measured and analysed carefully, it can be used to deduce the pathlength of the light wave inside the liquid." And indeed: irrespective of the number of nanoparticles, no matter whether the light was sent through an almost perfectly transparent sample or a milk-like liquid, the average path length of light was observed to be always the same.

This result helps to understand the propagation of waves in disordered media. There are many possible applications for this: "It is a universal law, which in principle holds for any kind of wave," says Stefan Rotter. "The same rules that apply to in an opaque also hold for sound waves, scattered at tiny objects in air or even gravity waves, travelling through a galaxy. The basic physics is always the same."

Explore further: The beam of invisibility

More information: Romolo Savo et al. Observation of mean path length invariance in light-scattering media, Science (2017). DOI: 10.1126/science.aan4054

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5 / 5 (1) Nov 10, 2017
One of those very nice results that could have been found 100 years ago or more
5 / 5 (4) Nov 10, 2017
One correction to the above article. At the end they reference 'gravity waves.' They clearly mean 'gravitational waves,' which do not have anything to do, directly, with the apparent force of gravity, but are changes in lengths and times that vary as the wave passes. Gravity waves, on the other hand, are waves on an ocean, for instance, where two fluids are in contact and the interface oscillates up and down
1 / 5 (1) Nov 12, 2017
ya kidding right? which charges are affected, i.e. is the container a restraint? Which locations have less restraint. Juz saying. Though we did this when we calculated a Gaussian Beam Moving through and Inhomogeneous Media. I did that for my BS in EE, jus say'n Shoulda went to T.
5 / 5 (1) Nov 13, 2017
BTW Wouldn't the mean path of light rays depend on the shape of vessel too? Try to imagine the passing of light through flat cuvette - every scattering would prolonge the mean path of light through it..
Every scattering? Imagine a scattering that occurs at the front of the cuvette that sends the light backwards, i.e. the light hardly enters before it bounces back out whence it came. That single counter-example falsifies your statement. In fact, the relative ratio of scatterings that are ~90 degrees to the initial path and hence liable to keep the photon in the cuvette are small compared to all the possible scattering angles.

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