Polarized neutron scattering reveals preferred spin excitations in bilayer iron-based superconductor

Polarized neutron scattering reveals preferred spin excitations in bilayer iron-based superconductor
(a) Mean-field phase diagram of the magnetic states in iron pnictides [15]. (b),(c) Phase diagram and SVC magnetic structure of CaK(Fe1−xNix)4As4. The arrow marks the doping in this study. (d) The scattering plane and the definition of spin-polarization directions in reciprocal space. (e) Schematic picture of the fluctuating moments under SVC order. Assuming M2 is fixed, M1 is allowed to fluctuate either transverse out of plane (Mc) or longitudinal in plane (Ma). (f) Magnetic order parameter at Q=(1,0,1) and (1, 0, 3) measured by polarized elastic neutron scattering. (g) Three components of static moments (open) in comparison with the unpolarized results (solid). Credit: Physical Review Letters (2022). DOI: 10.1103/PhysRevLett.128.137003

In unconventional superconductors, the major challenge on the mechanism research is to reveal how the electrons form to Cooper pairs and collectively condense to a superconducting state under both interactions from charge and spin. The iron-based superconductors are similar to those copper oxide and heavy fermion superconductors, and they also exhibit strong spin fluctuations, which likely promote the superconducting pairing by acting as the bosonic "pairing glue." Such argument is supported by a spin resonance mode with a peak energy universally linear scaling with Tc. However, it is still unknow whether in such multi-orbital systems the spin system may have some preferred fluctuating directions that is coupled to the orbital degree of freedom.

Neutron scattering is a direct probe to measure the spin fluctuations in materials, and thus a powerful tool in the mechanism research of unconventional superconductivity. With in polarized , it will give us detailed information about the spin-orbit coupling and the spin anisotropy in iron-based superconductors.

So far, there are three confirmed magnetic orders in iron pnictide superconductors: the collinear stripe-type order with in-plane moments so-called as stripe spin-density wave (SSDW); the collinear biaxial order with c-axis polarized moments so-called as charge-spin-density wave (CSDW); and the noncollinear, coplanar order with in-plane moments so-called as spin-vortex crystal (SVC) phase. Accumulating evidences suggest the spin resonance is preferentially polarized along c-axis in the superconducting state coexisting with the SSDW or CSDW orders.

Recently, Liu Chang et al. in Profs. Luo Huiqian and Li Shiliang's group from Institute of Physics of the Chinese Academy of Sciences (CAS), in collaboration with Bourges Philippe, Sidis Yvan from Universite Paris-Saclay, He Guanghong and Li Yuan from Peking University and other colleagues, have revealed the spin resonance mode and the spin anisotropy in the SVC ordered superconductor CaK(Fe0.96Ni0.04)4As4.

The researchers have discovered two spin resonance modes with odd and even L-symmetries with respect to the reduced distance within the Fe-As bilayer unit. Polarization analysis suggests that the odd mode is highly anisotropic, manifested by a strong c-axis component and two weakly anisotropic in-plane components. Such c-axis preferred spin excitations already show up in the SVC phase and even continue to the paramagnetic phase until the spin anisotropy finally disappears at high temperature.

These results provide the missing piece of the puzzle on the spin-orbit coupling effect in iron-pnictide superconductors, and suggest that the c-axis magnetic excitations are universally preferred by the presumably orbital-selective superconducting pairing.

Meanwhile, the form of magnetic order depends on material-specific symmetry characteristics in addition to , leading to a rich variety of interplay between superconductivity and magnetism in the iron-based superconductors.

This study was published in Physical Review Letters.


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More information: Chang Liu et al, Preferred Spin Excitations in the Bilayer Iron-Based Superconductor CaK(Fe0.96Ni0.04)4As4 with Spin-Vortex Crystal Order, Physical Review Letters (2022). DOI: 10.1103/PhysRevLett.128.137003
Journal information: Physical Review Letters

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