Design and validation of world-class multilayered thermal emitter using machine learning

March 15, 2019, National Institute for Materials Science
Schematic diagram showing the materials informatics method combining machine learning and the calculation of thermal emission properties and experiments conducted to verify the performance of fabricated materials. Credit: NIMS

NIMS, the University of Tokyo, Niigata University and RIKEN have jointly designed a multilayered metamaterial that realizes ultra-narrowband wavelength-selective thermal emission by combining the machine learning (Bayesian optimization) and thermal emission properties calculations (electromagnetic calculation). The joint team then experimentally fabricated the designed metamaterial and verified the performance. These results may facilitate the development of highly efficient energy devices.

Thermal radiation, a phenomenon that an object emits heat as electromagnetic waves, is potentially applicable to a variety of energy devices, such as wavelength-selective heaters, infrared sensors and thermophotovoltaic generators. Highly efficient thermal emitters need to exhibit with narrow bands in practically usable wavelength range.. The development of such efficient thermal emitters has been targeted by many researches using metamaterials that can manipulate electromagnetic waves. However, most of them have taken an approach of characterizing the material structures selected empirically, it has been difficult to identify the optimum structure from a vast number of candidates.

The joint research group developed a method of designing metamaterial structures with optimum thermal radiation performance using a combination of machine learning and the calculation of properties. This project focused on easy-to-fabricate multilayered metamaterial structures composed of three types of materials in 18 layers of varying thickness. Application of this method to about eight billion candidate structures led to the prediction that a nanostructure composed of non-periodically arranged semiconductor and dielectric materials would have superior performance, which was contrary to the conventional knowledge. Then the research group actually fabricated the metamaterial structure and measured its thermal spectrum, and consequently demonstrated an extremely narrow thermal emission band. Measured in terms of the Q-factor (a parameter used to measure the width of thermal emission spectral bands), the newly designed nanostructure produced a Q-factor close to 200, when 100 had been considered the upper limit for conventional materials—an exceptionally narrow thermal emission spectral band.

This research demonstrated the effectiveness of in developing highly efficient thermal emission metamaterials. The development of with desirable thermal emission spectra is expected to facilitate more efficient energy use throughout the society. Because the nanostructure design method developed is applicable to all kinds of materials, it may serve as an effective tool for the design of high-performance materials in the future.

This study was published in ACS Central Science.

Explore further: 'Thermal metamaterial' innovation could help bring waste-heat harvesting technology to power plants, factories

More information: Atsushi Sakurai et al, Ultranarrow-Band Wavelength-Selective Thermal Emission with Aperiodic Multilayered Metamaterials Designed by Bayesian Optimization, ACS Central Science (2019). DOI: 10.1021/acscentsci.8b00802

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