April 4, 2023

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New quantum sensing method holds promise for improving greenhouse gas detection

Schematic of the sensing strategy where a squeezed comb probes a gas with a frequency-dependent transmission η. The probe is generated by displacing a broadband squeezed vacuum state |ξ⟩ with a coherent state |α⟩ using a highly reflective beam splitter (BS) followed by a phase modulator (PM). The detection system consists of a balanced homodyne detector (HD) with a phase-tunable local oscillator (LO) followed by a spectrum analyzer (SA). Credit: Physical Review Letters (2023). DOI: 10.1103/PhysRevLett.130.133602
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Schematic of the sensing strategy where a squeezed comb probes a gas with a frequency-dependent transmission η. The probe is generated by displacing a broadband squeezed vacuum state |ξ⟩ with a coherent state |α⟩ using a highly reflective beam splitter (BS) followed by a phase modulator (PM). The detection system consists of a balanced homodyne detector (HD) with a phase-tunable local oscillator (LO) followed by a spectrum analyzer (SA). Credit: Physical Review Letters (2023). DOI: 10.1103/PhysRevLett.130.133602

An innovative new technique to detect and characterize molecules with greater precision has been proposed, paving the way for significant advances in environmental monitoring, medical diagnostics, and industrial processes.

The new quantum sensing method, put forward by a University of Bristol physicist, builds on the work of 2005 Nobel laureates in physics John Hall and Theodor Hänsch who developed a frequency comb technique to accurately measure optical frequencies. Frequency combs are deployed in many areas of science and industry to characterize matter based on the unique way light is absorbed.

However, the precision of optical comb spectroscopy is limited by a fundamental level of noise present in all lasers and other classical sources of light. A with reduced noise called "squeezed light" can overcome this limitation and has been harnessed to improve the sensitivity of gravitational wave detectors.

In a paper published in Physical Review Letters, squeezed light is shown to significantly suppress noise over a broad set of comb frequencies used to probe an absorbing molecule.

Author Alex Belsley, Quantum Engineering Ph.D. student, said, "This work proposes a new method for monitoring gas species in situ and with high precision. Quantum advantage in sensing can be realized today and I'm excited for the transformative impact quantum-enhanced sensors will have on our society in the coming years."

Illustration of an optical frequency comb probing gas molecules. Credit: Alex Belsley
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Illustration of an optical frequency comb probing gas molecules. Credit: Alex Belsley

This novel approach could potentially achieve more than a ten-fold improvement in detection limits. In addition to allowing different types of gases to be characterized at ultra-low concentrations, it can also determine important properties such as temperature and pressure with high sensitivity.

Professor Jonathan Matthews, co-director of the Quantum Engineering Technology Labs and Alex Belsley's Ph.D. advisor, said, "Better sensors are important to our future. Healthcare, manufacturing, and new science itself, all benefit from advances in how we measure physical properties. Alex's work shows how squeezed light can improve comb spectroscopy—the next step is to explore further with experiments in the lab."

More information: Alexandre Belsley, Quantum-Enhanced Absorption Spectroscopy with Bright Squeezed Frequency Combs, Physical Review Letters (2023). DOI: 10.1103/PhysRevLett.130.133602

Journal information: Physical Review Letters

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