October 24, 2019

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Flexible, transparent and cost-effective lasers

Three distributed feedback structures illuminated by an UV lamp. Credit: Juan Cabanillas-González
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Three distributed feedback structures illuminated by an UV lamp. Credit: Juan Cabanillas-González

The interest in plastic electronics and photonics has experienced a significant increase in the last decades due to the exceptional optical, semiconducting and mechanical properties of these materials. Plastic electronics, based on conjugated polymers, combine the benefits of cost-effective processability compatible with large-area deposition for designing laser geometries of virtually any shape. This is impossible with rigid inorganic semiconductor materials. These highly luminescent materials have been incorporated into a variety of resonator geometries such as photonic crystals or distributed feedback (DBF) cavities to enable optically pumped conjugated polymer lasers with emission across the visible and near-infrared spectrum.

A between IMDEA Nanociencia and Nanjing Tech University researchers has produced novel transparent, all-polymer DBF lasers. The DBF lasers make use of the periodic wavelength-scale nanostructures to backscatter photons for constructive interference. In their work, DBF structures were nanoimprinted on thermoplastic (cellulose diacetate) films and covered by highly luminescent conjugated polymers. In this way, the designed lasers present a homogeneous emission in the blue, green and red colors. Additionally, the emission wavelength is tunable by bending the DBF flexible cavities.

The advantages of using thermoplastic materials such as cellulose diacetate as substrates are many: It is cheap, readily available, flexible and transparent, even upon annealing. Also, cellulose diacetate is compatible with several , it is obtained from renewable wood pulp, and it is biodegradable. Researchers have demonstrated the robustness of their structures by assessing the lasing threshold values upon bending, confirming that the optical and structural properties of the active layer do not deteriorate.

The followed strategy is scalable and versatile. DBF lasers have currently a wide range of applications as mechanically flexible lasers, for instance, on lab-on-a-chip devices in biomedical analysis, information technology and sensing.

More information: José R. Castro Smirnov et al. Flexible distributed feedback lasers based on nanoimprinted cellulose diacetate with efficient multiple wavelength lasing, npj Flexible Electronics (2019). DOI: 10.1038/s41528-019-0062-4

Provided by IMDEA Nanociencia

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