Heavy fermions get nuclear boost on way to superconductivity

Heavy fermions get nuclear boost on way to superconductivity
This microscopic closeup shows a small sample of ytterbium dirhodium disilicide, one of the most-studied 'heavy fermion' composites. The scale bar in the center of the screen is one millimeter wide. Credit: Marc Tippmann/Technical University of Munich

In a surprising find, physicists from the United States, Germany and China have discovered that nuclear effects help bring about superconductivity in ytterbium dirhodium disilicide (YRS), one of the most-studied materials in a class of quantum critical compounds known as "heavy fermions."

The discovery, which is described in this week's issue of Science, marks the first time that has been observed in YRS, a composite material that physicists have studied for more than a decade in an effort to probe the quantum effects believed to underlie .

Rice University physicist and study co-author Qimiao Si said the research provides further evidence that arises from "quantum criticality."

"There is already compelling evidence that unconventional superconductivity is linked in both copper-based and iron-based high-temperature superconductors to quantum fluctuations that alter the magnetic order of the materials at 'quantum critical points,' watershed thresholds that mark the transition from one quantum phase to another," Si said. "This work provides the first evidence that similar processes bring about superconductivity in the canonical heavy-fermion system YRS."

Electrons fall within a quantum category called fermions. Heavy fermions are composite materials that contain rare earth elements. Their name stems from the fact that at extremely low temperatures, typically less than 1 kelvin, electrons move through the material as if they were 1,000 times more massive than normal. In the latest experiments, Si said, the measured heat capacity was so large that the electrons behaved as if they were heavier still—about 1 million times heavier than normal. This occurred as the YRS was cooled to just above the point of superconductivity, around 2 millikelvins.

Heavy fermions get nuclear boost on way to superconductivity
Erwin Schuberth (left) and Marc Tippmann with a high-performance cryostat at the Walther Meissner Institute in Garching, Germany. Credit: Andreas Battenberg/Technical University of Munich

Si, Rice's Harry C. and Olga K. Wiess Professor of Physics and Astronomy. also directs the Rice Center for Quantum Materials (RCQM). He said the research was conducted in collaboration with RCQM partners in Germany and China. Experiments were performed at the Walther Meissner Institute for Low Temperature Research at the Bavarian Academy of Sciences in Garching, Germany, and at the Max Planck Institute for Chemical Physics of Solids in Dresden, Germany. Theoretical work was performed at Rice and at Renmin University of China in Beijing.

Experiments overseen by the Meissner Institute's Erwin Schuberth and the Max Planck Institute's Frank Steglich offered the first glimpse of YRS' behavior at the quantum critical point. Schuberth, who has appointments at both institutes as well as the Technical University of Munich, said what appeared to be an increase in apparent mass was actually the clue that nuclear forces were at work.

"Nothing else could have accounted for such a large change," he said.

The bulk of experiments were performed in Garching, where Schuberth's team used "adiabatic magnetic cooling" and other specialized techniques to make its YRS samples ultracold, about 10 times colder than those in any previous YRS experiment; this is what allowed the team to discover superconductivity.

In analyzing the evidence, Si and fellow theorist Rong Yu of Renmin University found that the arrangement of inertial spins of the ytterbium nuclei in the YRS composite helped bring about superconductivity. He said the nuclear spins became coupled at extremely low temperatures and arranged in an ordered pattern that exposed the quantum criticality of the electrons.

"In YRS, the spins of electrons are locked in a pattern that varies periodically in space and is the hallmark of an electronic order known as anti-ferromagnetism," Si said. "An ordered arrangement of the nuclear spins acts to suppress the electronic order, and this exposes the electronic quantum criticality, which in turn drives unconventional superconductivity."

The discovery of superconductivity in YRS followed a search lasting more than a decade. Steglich said the previous experiments demonstrate that quantum criticality in YRS brings electrons to the verge of being both localized and itinerant, a condition that was predicted by Si and collaborators in a landmark 2001 theory.

Steglich said, "In previous experiments, an external magnetic field revealed a quantum critical point with a host of truly remarkable electronic properties that had been predicted by theory. But the magnetic field also created a condition that is inhospitable to superconductivity."

The current work succeeded in discovering superconductivity by reaching quantum criticality through the ordering of nuclear spins at ultralow temperatures, without applying an .

"It is remarkable that it takes an act of to produce quantum criticality at zero and realize superconductivity," Steglich said.

Si said the new findings are important for the study of both heavy-fermion superconductivity and, more generally, the physics of quantum criticality.

"The work demonstrates that is a robust mechanism for bringing about unconventional superconductivity, not only in high-temperature superconductors, as had previously been shown, but also in heavy-fermion materials that are the canonical example of quantum critical behavior in every other respect," Si said.

Explore further

Evidence mounts for quantum criticality theory

More information: Emergence of superconductivity in the canonical heavy-electron metal YbRh2Si2, Science, DOI: 10.1126/science.aaa9733
Journal information: Science

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Jan 28, 2016
In Jan 2014, RBL introduced In "On the Mechanism of Above Room Temperature Superconductivity and Superfluidity by Relativistic Quantum Mechanics" {http://arxiv.org/abs/1412.4012 } the affect of nuclear spin (for the first time) as another type of magnetic interaction for modulating high temperature superconductivity of electron fermions via triple of spins involving electron spin pair (boson) and nuclear lone spin (fermion) for the nuclear spin magnetically modulating the bosonic superconducting electron pairs for loss of phonon scattering by the nuclei as the fermionic magnetic spins of the nuclei nondissipatively rotate the electron pair in nondissipative current! Scientists at US, Chinese and German Laboratories in Jan 2016 experimentally and computationally report the observation of such theory of RBL from Jan 2014!

Jan 28, 2016
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Jan 29, 2016
"Heavy fermions are composite materials that contain rare earth elements." Now, I'm not a rocket surgeon, but I'm going to say I'm about 97% sure that's completely wrong.

Jan 29, 2016
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Jan 29, 2016
This is another example of Art Winfree's law of coupled periodic oscillators. Specifically:

..."the nuclear spins became coupled at extremely low temperatures and arranged in an ordered pattern..."

Spins are a periodic oscillation. Art Winfree's law says that periodic oscillators have a tendency to couple. When they do, they will arrange in certain patterns, which he specified. He did not apply his law to physics-- he was a bio mathematician. I believe his law applies extensively to physics.

See my many prior Physorg posts for info about Winfree's law and its application to physics, including all forms of superconductivity.

Jan 29, 2016
Continuing my comment above, the nuclear spins organize pursuant to Winfree's law.

Now let's focus on the arrangement of the electrons. How do they organize into Cooper pairs and become superconducting? IMO they also organize pursuant to Winfree's law. Cooper pairs are a Winfree pattern. They couple anti-synchronously by orbit, and anti-synchronously by spin (one up, the other down). Orbits and spins are periodic oscillations.

Returning now to the nuclear spins, how does their organization (by Winfree's law) promote the organization of electrons into Cooper pairs (by Winfree's law)? Ordered nuclear arrangements will produce more stable, precise and orderly oscillations of the electrons. That permits this rare Winfree organization (otherwise known as Cooper pairs) of the electrons.

Anti-ferromagnetic order, mentioned in the article, is also a Winfree pattern--just not a superconducting Winfree pattern, as BCS Cooper pairs are.

Jan 30, 2016
If the opposite pointing spin patterns of electrons or protons is requirement for superconductivity, it explains why external or current generated magnetic field does destroy this order and therefore superconductivity.

Feb 01, 2016
If the opposite pointing spin patterns of electrons or protons is requirement for superconductivity, it explains why external or current generated magnetic field does destroy this order and therefore superconductivity.

There are critical magnetic field and current strengths. When these are exceeded superconductivity is destroyed.

Thanks, that was what I meant to write, that with strong enough magnetic field the superconductivity is not possible. And what is strong enough depends on materials and temperatures.

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