Water bottles, other recycled 3-D printing materials could avoid military supply snags

August 21, 2018, American Chemical Society
With 3D-printers, soldiers could soon use recycled bottles and other waste materials to make vital parts, such as this vehicle radio bracket. Credit: Nicole Zander/U.S. Army Research Laboratory

Soldiers on the battlefield or at remote bases often have to wait weeks for vital replacement parts. Now scientists report they have found a way to fabricate many of these parts within hours under combat conditions using water bottles, cardboard and other recyclable materials found on base as starting materials for 3-D printing. They say this 'game-changing' advance could improve operational readiness, reduce dependence on outside supply chains and enhance safety.

The researchers are presenting their work today at the 256th National Meeting & Exposition of the American Chemical Society (ACS).

"Ideally, soldiers wouldn't have to wait for the next supply truck to receive vital equipment," Nicole Zander, Ph.D., says. "Instead, they could basically go into the cafeteria, gather discarded water bottles, milk jugs, cardboard boxes and other recyclable items, then use those materials as feedstocks for 3-D printers to make tools, parts and other gadgets."

Supplying combat troops with food, fuel, ammunition and repair parts is a monumental task, requiring thousands of support staff, contractors and manufacturers. In all, the U.S. Department of Defense has an inventory of 5 million items distributed through eight distinct supply chains, according to the U.S. Government Accountability Office. However, few of these items are stockpiled at front-line locations, meaning that troops in those areas can experience occasional shortages of important materials. Many of these units have 3-D printers that can produce spare parts and other equipment, but they rely on conventional feedstocks, such as commercially available filaments, that must be requisitioned, and they can take days, weeks or even months to arrive.

Recently, Zander, U.S. Marine Corps Capt. Anthony Molnar and colleagues at the U.S. Army Research Laboratory explored the possibility of using recycled polyethylene terephthalate (PET) plastic as a starting material for 3-D printers. PET plastics, found in water and soda bottles, are common waste materials found around bases, and the researchers realized that this material could be a viable feedstock. They determined that PET filaments, produced by recycling, were just as strong and flexible as commercially available filaments for 3-D printers. In tests, the team used recycled PET filaments to print a vehicle radio bracket, a long-lead-time military part. This process required about 10 and took about two hours to complete.

Initially, the researchers determined that other types of plastic, such as polypropylene (PP), used in yogurt or cottage cheese containers, or polystyrene (PS), used for plastic utensils, were not practical for use in 3-D printing. Undeterred, the team sought to strengthen PP by mixing it with cardboard, wood fibers and other cellulose waste materials found on military bases to create new composite filaments. In addition, the very brittle PS was blended with ductile PP to generate a strong and flexible .

The researchers used a process called solid-state shear pulverization to generate composite PP/cellulose filaments. In this process, shredded plastic and paper, cardboard or wood flour was pulverized in a twin-screw extruder to generate a fine powder that was then melt-processed into 3-D printing filaments. After testing using dynamic mechanical analysis, the scientists concluded that the new composites had improved mechanical properties, and they could be used to make strong 3-D-printed materials.

Zander's team is building a mobile recycling trailer that will enable specially trained soldiers to fabricate 3-D-printing filaments from plastic waste. She is also exploring ways to print materials from plastic pellets instead of filaments, which could help soldiers quickly produce larger 3-D-printed parts and machinery.

"We still have a lot to learn about how to best process these and what kinds of additives will improve their properties," Zander says. "We're just scratching the surface of what we can ultimately do with these discarded plastics."

Explore further: Improving 3-D printing of plastic parts

More information: 3D Printing Feedstocks from Recycled Materials, the 256th National Meeting & Exposition of the American Chemical Society (ACS).

Abstract
United States warfighters in theater are often faced with the challenge of broken, damaged, or missing parts necessary to maintain the safety and productivity required. Waste plastics can be utilized to improve the self-reliance of warfighters on forward operating bases by cutting costs and decreasing the demand for the frequent resupplying of parts by the supply chain. In addition, the use of waste materials in additive manufacturing in the private sector would reduce cost and increase sustainability, providing a high-value output for used plastics. Experimentation is conducted to turn waste plastics filament that can be used in fused filament fabrication. The effect of extrusion temperature and number of extrusion cycles on polymer viscosity and crystallinity are explored. The effect of blends and fillers to impart additional functionality are also examined. Tensile specimens were tested and compared to die-cut and injection molded parts. Parts printed from recycled polyethylene terephthalate had the highest tensile strength of all recycled plastics evaluated (35.1 ± 8 MPa), and were comparable to parts printed from commercial polycarbonate-ABS filament. Elongation to failure of all recycled plastics was similar to their injection molded counterpart. In addition, select military parts were printed with recycled filament and compared to original parts. This research demonstrates some of the first work on the feasibility of using recycled plastic in additive manufacturing.

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