Uncovering the secrets of spin-orbit optical Rabi oscillations

So far only two independent classes of wave states in the Rabi oscillations have been revealed as and orbital waves, while a Rabi wave state simultaneously merging the spin and orbital angular has remained elusive.

In a new paper published in Light: Science & Applications, a team of scientists, led by Professor Zhen Li and Shenhe Fu from Department of Optoelectronic Engineering, Jinan University, China, and co-workers have reported a new form of Rabi oscillation, exhibiting both spin and orbital angular momentum.

To reveal this fundamental phenomenon, they constituted a pseudo spin-1/2 formalism and optically synthesized a controllable magnetic field in the light-crystal interaction process. Based on this formulism, they observed simultaneous oscillations of the spin and orbital angular momentum in weak and strong coupling regimes, driven by the beam-dependent synthetic magnetic field.

Furthermore, they introduced an electrically tunable platform, allowing a fine control of transition between different Rabi oscillatory modes, resulting in an emission of orbital-angular-momentum beams with tunable topological structures. Their results constitute a general framework to explore spin-orbit couplings in the higher-order regime, offering routes to manipulating the spin and orbital angular momentum of light in three and four dimensions. The reported method and technique will find potential applications both in classical and .

a, The original spin-1/2 setting describing spinnings of a quantum particle in a driven magnetic field, where the spin up and spin down constitute the two-level eigenstates. b, In the presented setting, the eigenstates R and L simultaneously coupling with the SAM and OAM are defined as the spin up and spin down equivalents, respectively. These pseudo spin up and spin down states are coupled by a synthetic magnetic field. c, The higher-order Poincaré sphere is introduced to represent the spin-orbit states, with two poles denoting the eigenstates. d, Typical states mapped on the sphere (marked points in c) showing spatial variations of polarization (upper panels) and phase (bottom panels) distributions with polar angle. The arrows in the upper panels denote polarizations; while the black lines in the bottom panels represent the phase contours. Credit: Guohua Liu, Xiliang Zhang, Xin Zhang, Yanwen Hu, Zhen Li, Zhenqiang Chen, and Shenhe Fu

a, b, The electrically tunable synthetic magnetic field allows Rabi transition between different oscillatory modes: a, V = ±50 V (trajectories in blue and purple); b, V = ±200 V (trajectories in blue and purple). c, The spinor moves slowly from point A to its initial position by gradually sweeping the voltage from 0 to 1000 V, see blue curve; while altering the voltage sign producing a symmetric trajectory (purple line). d, The same as described in c but in a different case of beam width. e, f, The emitted topological charge as a function of voltage after a coupling length z =30 mm, in two different cases of beam widths. Credit: Guohua Liu, Xiliang Zhang, Xin Zhang, Yanwen Hu, Zhen Li, Zhenqiang Chen, and Shenhe Fu

The Rabi oscillation is manifested partially by the separated orbital-angular-momentum oscillation along with the coupling length. a, b, The interferograms recorded at different coupling lengths: a, experiments; b, simulations. c, Simulated phase distributions of light fields at the corresponding coupling lengths. Credit: Guohua Liu, Xiliang Zhang, Xin Zhang, Yanwen Hu, Zhen Li, Zhenqiang Chen, and Shenhe Fu