Spontaneous decays of magneto-elastic excitations in non-collinear antiferromagnets

It's official: Phonon and magnon are a couple
Good match between the results of the neutron scattering experiments (top) and the theoretical model (bottom). Credit: IBS, Nature Comms

Professor Park Je-Geun of the Institute for Basic Science (IBS) and colleagues have created a new theoretical model of the coupling of two forms of collective atomic excitation, known as magnons and phonons in crystals of the antiferromagnet manganite (Y,Lu)MnO3, a mineral made of manganese oxide and the rare-earth elements yttrium (Y) and lutetium (Lu).

This study could provide an important breakthrough for solving a 100-year-old physical problem, and deepen our knowledge of an interesting class of materials called multiferroics. The complete theoretical model and experimental observations can be read on Nature Communications.

While we generally think of solids as static objects, their molecules are actually in a constant state of vibration. These small vibrations are partly due to and magnons, which are collective excitations and disturbances inside a crystal. Collective means that they are not limited to a single atom, but influence a group of neighbouring atoms. Phonons are uniform oscillations at a single frequency. For example, short-wavelength phonons play a role in thermic conduction, while long-wavelength phonons give rise to sound, which is the origin of the word ("phonos" means voice in Greek). Magnons are collective perturbations of the electrons' spins, the compasses of the atoms. They influence the magnetic characteristics of the materials. This report shows, for the first time, that the two couple, and as a consequence, their vibratory behavior is not constant over time.

IBS scientists measured the atomic and molecular motion of (Y,Lu)MnO3 crystals by inelastic neutron scattering experiments and also derived a new theoretical model to explain what they observed experimentally. Interestingly, they had to go beyond the standard linear theory, which is normally used to interpret the measurements. The standard linear spin wave theory presumes that the vibration of magnons and phonons is harmonic and stable over time, like the oscillation of a spring without friction. "Initially, we used the simplest model, which is the linear spin wave theory without a coupling, but we realised that it was like the classic case of putting the elephant in the fridge: You can manage it, but the numbers become unrealistic and there is something wrong with it," explains professor Park Je-Geun. "Then we did the calculations again, this time including the coupling, and we discovered that we could explain the data and, most importantly, the final analysis gave us numbers that make sense."

The animation is a simplified way to represent the vibration that occurs inside the solids and illustrates how phonons and magnons are interrelated. Phonons are the waves that make the molecules (circles) oscillate, while the magnons are shown as the movement of compass-like arrows (spins). The animation shows that the wave created by the phonons make the spins move and vice versa. While the standard linear spin wave theory says that this collective movement can last forever, this new research shows that phonons and magnons influence each other by coupling, and this collective movement is not stable. Credit: Park Je-Geun, IBS

While the standard linear spin wave theory says that magnons and phonons vibrate forever and do not influence each other, a coupling would make phonons and magnons unstable, and allow an otherwise forbidden decay.

"The idea of a magnon-phonon coupling has already been around as a possible explanation for the uniquely low coefficient of thermal expansion of the invar materials. These industrially important materials have a range of uses from Swiss watches to high-speed trains, but why these materials exhibit such a counterintuitive behavior has been a puzzle for many decades," says the professor.

While the coupling was rarely observed before, this is the first time that it has been quantified in manganite crystal: "It is a weak coupling, and present only in some materials, because it needs a particular triangular atomic architecture. It also conflicts with the mainstream belief that magnons and phonons are stable over time. This could explain why the coupling has never been carefully analyzed before, and why most scientists have ignored it," says the professor.

In the future, the team would like to study this coupling in other materials and ideally demonstrate that one can artificially convert phonons into magnons and vice versa.


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More information: Joosung Oh et al, Spontaneous decays of magneto-elastic excitations in non-collinear antiferromagnet (Y,Lu)MnO3, Nature Communications (2016). DOI: 10.1038/ncomms13146
Journal information: Nature Communications

Citation: Spontaneous decays of magneto-elastic excitations in non-collinear antiferromagnets (2016, October 19) retrieved 27 May 2019 from https://phys.org/news/2016-10-spontaneous-magneto-elastic-non-collinear-antiferromagnets.html
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Oct 19, 2016
Good work. This is consistent with my theory of coupled oscillators that I have explained and applied in many Physorg posts. Google Macksb Physorg Winfree for more info about my theory and its many applications. My theory derives from Huygens and Art Winfree.

Periodic oscillations include a wide range of motions, from vibrations to quanta. Per the article, phonons are uniform periodic oscillations at a single frequency. That is why they couple collectively. Also per the article, magnons are collective perturbations of electron spins. As you can see in the video, the spin arrows oscillate periodically left and right, anti-aligned with their immediate neighbors. These oscillations can also couple widely into a single (uniform) frequency as well

Since the phonons and the magnons influence each other, the phonon group and the magnon group are likely to couple their group level periodic oscillations. Just like Huygens' pendulum clocks 350 years ago.

Oct 19, 2016
Notice the need for a "particular triangular atomic architecture." See the penultimate paragraph in the Physorg article.

To understand this better, see the large (and complex) diagram in the full article as published in Nature Communications. To get there (free) just click on the black bold DOI section at the very end of the above Physorg article.

When you get to the Nature Communication article you will see triangles and the atomic architecture in the upper left hand diagram or illustration. Within that particular diagram of triangles you will see three small, red spin arrows in the lowest triangle. This will give you a good visual understanding of what the particular triangular architecture looks like. And with some imagination, you can see why any two of those spin arrows would oscillate in a cycle that is counter to the cycle of its nearest neighbor spin arrow.

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