Using laser beams, scientists generate quantum matter with novel, crystal-like properties

November 1, 2012 by Olivia Meyer-streng, Max Planck Society

Using laser beams, scientists generate quantum matter with novel, crystal-like properties
Figure 1: Illustration of an ordering of five Rydberg-atoms. Green: atoms in the ground state. Red: Rydberg-atoms. Violet: Sphere of influence of the Rydberg-atoms.
(—Both high-valued diamond and low-prized graphite consist of exactly the same carbon atoms. The subtle but nevertheless important difference between the two materials is the geometrical configuration of their building blocks, with large consequences for their properties. There is no way, any kind of matter could be diamond and graphite at the same time.

However, this limitation does not hold for , as a team of the Quantum Many-Body Physics Division of Prof. Immanuel Bloch (Max-Planck-Institute of and Ludwig-Maximilians-Universität München) was now able to demonstrate in experiments with ultracold quantum gases. Under the influence of single atoms would arrange to clear geometrical structures (Nature, November 1st, 2012). But in contrast to classical crystals all possible configurations would exist at the same time, similar to the situation of Schrödinger's cat which is in a superposition state of both "dead" and "alive". The observation was made after transferring the particles to a highly excited so-called Rydberg-state. "Our experiment demonstrates the potential of Rydberg gases to realise exotic states of matter, thereby laying the basis for quantum simulations of, for example, quantum magnets," Professor Immanuel Bloch points out. The experimental work was supported by theoretical performed in the group of Dr. Thomas Pohl (Max Planck Institute for the Physics of Complex Systems, Dresden). 

The experiment begins with cooling an ensemble of a couple of hundred down to temperatures near and catching the atoms in a . The atomic cloud is then superimposed with a periodic light field – a so-called which provides an almost uniform filling in the central area of the trap. In the next step laser light is applied to transfer the atoms into a Rydberg-state in which the outermost shell electron is at a fairly large distance from the atomic nucleus. As a result, the sphere of influence of these atoms is blown up, like a balloon, by a factor of about 10 000, reaching a comparatively "huge" diameter of several micrometres – this is more or less equivalent to the tenth part of the diameter of an average hair. These super-atoms now interact strongly via so-called van der Waals forces, which act on the same range.

As the scientists chose Rydberg-states which give rise to repulsive van der Waals forces the excited atoms have to keep a minimum distance of several micrometers from each other. This mutual blockade leads to spatial correlations between the atoms such that, depending on the number of Rydberg-atoms, states with different geometrical configurations can emerge (see fig. 1). "However, we have to be aware that in our excited quantum system all geometrical orders are present at the same time. To be precise, all the excitation states form a coherent superposition," Dr. Marc Cheneau says, a scientist at the experiment. "This new state of matter is a very fragile, crystal-like formation; it exists as long as the excitation is sustained, and fades away once the beam is switched off."

Figure 2: Different geometrical configurations of selected excitation states. a) Single snapshots of excitations states with a different number of Rydberg-atoms; b) Resulting patterns after grouping many individual images according to the number of Rydberg-atoms; c) Results of the numerical calculations

As soon as the system undergoes an observation the superposition decays into a specific excitation state, with a certain number of Rydberg-atoms in a certain configuration (this is again in analogy to the example of Schrödinger's cat which is found, once it is looked after, either dead or alive). In a series of "snap shots" the scientists discover the different patterns of the individual excitation states. This is possible by using a special technique which images each Rydberg-atom directly by its fluorescence light, with very high spatial resolution. "We observe the emergence of spatially ordered excitation patterns with random orientation, but a well defined geometry," Peter Schauß explains, who works at the experiment as a doctoral candidate. In order to recognize the fundamental structures the individual images are grouped according to the number of Rydberg-atoms. Typical microscopic configurations are shown in figure 2. Three atoms are arranged on an equilateral triangle, four or five atoms form quadratic or pentagonal configurations. The experimental data was in good agreement with numerical simulations of the many-body dynamics which were performed by the group of Dr. Thomas Pohl.

As far as the pattern of each individual excitation state is concerned the observations can be described classically. "In order to reveal the quantum physical behaviour of our system we investigate the time-dependent probabilities for the different excitation states, each characterized by a certain number of Rydberg-atoms," Peter Schauß says "Thereby we were able to discover that the dynamic of the excitation process is ten times as fast as in classical systems without blockade effects. This is a first indication that our system is indeed a coherent quantum state, composed of different spatially ordered configurations." 

A future challenge for the scientists is the deterministic preparation of Rydberg crystals with a well defined number of excitations. Combining the blockade effect with the single-atom addressing one could engineer quantum gates which can serve as an experimental toolbox for a variety of . Several Rydberg-atoms could be connected to a scalable quantum system for quantum information processing.

Explore further: Giant Rydberg atoms confined in a micro-glass cell

More information: Schaub, P. et al., Observation of spatially ordered structures in a two-dimensional Rydberg gas. Nature, November 1st, 2012.

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3 / 5 (2) Nov 01, 2012
There is some historical precedent. Circa 1967, Art Winfree (who won the MacArthur prize many years later) described a law of coupled oscillators. A system of periodic oscillators will have certain predictable stable patterns. One of those systems is each piece one-third out of phase to its neighbors. Or one-fourth out of phase. Or one-fifth out of phase. That is the result obtained above, most clearly visible in C. Art Winfree described himself as a biomathematician, so he is not widely known in physics.
1 / 5 (1) Nov 04, 2012
Consider the implications of my post above.

1. Winfree's law of coupled oscillators is the theoretical explanation for the result described in this article. The pattern match is not coincidental. Winfree's theory applies generally to periodic oscillations of all types. Planck's quantum of energy is a periodic oscillation.

2. If that proposition is true, Winfree's law is the theoretical explanation for all phases of matter and their transitions: solid, liquid, gas, plasma; superconductivity (all types)and superfluidity; and the various new quantum phases of matter. This Rydberg state is "crystal-like." One principle--Occam.

3. Take the number of units (3, 4 or 5 in the above example) and divide into 360 (the unit of periodicity). That's quantum geometry for coherent systems of periodic oscillators. Same rule for spin waves. Complex oscillator systems with different oscillators and a variety of oscillations give us the periodic table of the elements.

Critics may fire when ready.

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