Electronic 'crowd behavior' revealed in semiconductors

Jul 07, 2007
Electronic 'crowd behavior' revealed in semiconductors
Physicists at JILA have confirmed subtle "collective behavior" among electronic structures in semiconductors, research that may help improve the design of optoelectronic devices. In the first image (#1, showing new experimental data), matching large peaks in the foreground, showing energy intensity ranging from low in blue to high in red, indicate that pairs of large electronic particles called excitons are oscillating in concert as they absorb ultrafast laser light and emit energy at various frequencies. The data match new theoretical models accounting for all electronic properties of semiconductors (image #2) much better than older theoretical models. Credit: JILA and University of Marburg

Like crowds of people, microscopic particles can act in concert under the right conditions. By exposing crowd behavior at the atomic scale, scientists discover new states and properties of matter.

Now, ultrafast lasers have revealed a previously unseen type of collective electronic behavior in semiconductors, which may help in the design of optoelectronic devices. The work at JILA, a joint venture of the National Institute of Standards and Technology (NIST) and the University of Colorado at Boulder, is described in a new paper in the Proceedings of the National Academy of Sciences.

Electronic 'crowd behavior' revealed in semiconductors
Physicists at JILA have confirmed subtle "collective behavior" among electronic structures in semiconductors, research that may help improve the design of optoelectronic devices. Credit: JILA and University of Marburg

Design of optoelectronic devices, like the semiconductor diode lasers used in telecommunications, currently involves a lot of trial and error. A designer trying to use basic theory to calculate the characteristics of a new diode laser will be off by a significant amount because of subtle interactions in the semiconductor that could not be detected until recently.

To shed light on these interactions, the JILA team used a highly sensitive and increasingly popular method of manipulating laser light energy and phase (the point in time when a single light wave begins) to reveal the collective behavior of electronic particles that shift the phase of any deflected light. Their work is an adaptation of a technique that was developed years ago by other researchers to probe correlations between spinning nuclei as an indicator of molecular structure (and led to a Nobel prize).

In the latest JILA experiments, a sample made of thin layers of gallium arsenide was hit with a continuous series of three near-infrared laser pulses lasting just 100 femtoseconds each. Trillions of electronic structures called excitons were formed. Excitons are large, fluffy particles consisting of excited electrons and the “holes” they left behind as they jumped to higher-energy vibration patterns.

By tinkering with the laser tuning—the frequency and orientation of the electric field—and analyzing how the semiconductor altered the intensity and phase of the light, the researchers identified a subtle coupling between pairs of excitons with different energy levels, or electron masses. The experimental data matched advanced theoretical calculations of the electronic properties of semiconductors, confirming the importance of the collective exciton behavior—and dramatically demonstrated the superiority of those calculations over simpler models of semiconductor behavior (see graphic).

Citation: T. Zhang, I. Kuznetsova, T. Meier, X. Li, R.P. Mirin, P. Thomas and S.T. Cundiff. Polarization-dependent optical two-dimensional Fourier transform spectroscopy of semiconductors. Proceedings of the National Academy of Sciences. Scheduled to be posted on-line July 6.


Source: National Institute of Standards and Technology

Explore further: Experiment with speeding ions verifies relativistic time dilation to new level of precision

add to favorites email to friend print save as pdf

Related Stories

Twisted graphene chills out

1 hour ago

(Phys.org) —When two sheets of graphene are stacked in a special way, it is possible to cool down the graphene with a laser instead of heating it up, University of Manchester researchers have shown.

For electronics beyond silicon, a new contender emerges

18 hours ago

Silicon has few serious competitors as the material of choice in the electronics industry. Yet transistors, the switchable valves that control the flow of electrons in a circuit, cannot simply keep shrinking ...

Study sheds new light on why batteries go bad

Sep 14, 2014

A comprehensive look at how tiny particles in a lithium ion battery electrode behave shows that rapid-charging the battery and using it to do high-power, rapidly draining work may not be as damaging as researchers ...

Recommended for you

How Paramecium protozoa claw their way to the top

Sep 19, 2014

The ability to swim upwards – towards the sun and food supplies – is vital for many aquatic microorganisms. Exactly how they are able to differentiate between above and below in often murky waters is ...

User comments : 0